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Magneto. Would be cool if there was standalone game for a villain and especially Magneto. To be able to manipulate your environment would be cool to play.
The Punisher (rated M). Guest appearances by Spider-Man and daredevil (who may assist you or try to stop you depending on your choices throughout the game).
Mystique. This could be a cool āhit manā style stealth game where she infiltrates facilities, talks her way out of situations, then sabotages, steals, or causes distrust. It could take place in the marvel u so it could have other characters in it.
Bailey Hoskins. He could detonate himself, but doing so would would kill him. Struggle the entire game and then defeat the final boss and save the world sacrificially .